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Core-Shell Nanoparticles: Preparation and the Encapsulation and Release of Drugs
Author: WuLiLi
Tutor: ZhuXiaoLi
School: Jinan University
Course: Polymer Chemistry and Physics
Keywords: Casein Methyl methacrylate Butyl acrylate Graft polymerization Core - shell nanospheres
CLC: TQ460.1
Type: Master's thesis
Year: 2011
Downloads: 43
Quote: 0
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Abstract
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In this thesis, the emulsion polymerization process and is not using any emulsifiers and stabilizers used in the presence of t - butyl hydrogen peroxide (TBHP) , casein (CA) of methyl methacrylate (MMA) and acrylic acid as initiator, respectively butylacrylate (BA) in the CA on the graft polymerization, a diameter of about 150 nm having a core - shell structure of the PMMA / CA PBA / CA nano composite latex particles were prepared . Characterized by TEM results confirm a core-shell structure of the latex particles , the cores were hydrophobic PMMA, PBA, the housing for the hydrophilicity of the CA . Using laser particle size analyzer to test the particle size and size distribution of the latex particles , chloroform as solvent using Soxhlet extraction test grafting efficiency of PMMA, PBA . The effects of reaction temperature, and the amount of initiator and core-shell raw material quality than , the the materials total concentration of monomer conversion , grafting efficiency of PMMA and PBA , latex particle size and its distribution impact . Preparation of PMMA / CA core - shell nanoparticles , the monomer conversion and the latex particle size with reaction time changes in the experimental results show that : the beginning of the polymerization of 20 min , the latex particle suddenly reduced and then remained unchanged for 30 min single body conversion rate of 70 % to 73% within 3 h . When MMA conversion rate in the temperature controlled at 70 ℃ and 80 ° C , of TBHP dosage control in CA quality of 0.18% to 0.36 % , the the MMA / CA mass ratio of 4 , the total concentration of materials does not exceed 10 % of the conditions of grafting efficiency and PMMA higher than 75 % . CA - MMA total content reached 30% , the gel , this is because the shell of the latex particles is hydrophilic CA , contains a large amount of the amino group, a hydroxyl group and a carboxyl group , with water to form a strong hydrogen bonding interactions , with the system the CA content increases , the viscosity of the system increases rapidly. Preparation of PBA / CA when the core - shell nanoparticles experimental results show a clear core-shell : BA / CA mass ratio of 4, TBHP attributable CA quality of 0.22 % , the total content of Ca and BA in 10 % , 75 ° C the reaction can be obtained the structure of the latex particle, and can obtain higher monomer conversion rate and PBA graft efficiency . Thereafter continue to improve any of the above experimental parameters are the conversion rate of the BA , the grafting efficiency of the PBA , latex particle size distribution, etc. have a negative impact . The core-shell emulsion prepared dialysis using gas chromatography detection of residual monomer , and then use the the ultrasound law or oscillation prepared load paclitaxel core-shell particles of paclitaxel in the core-shell particles coated .
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