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Studies on Soft Cluster Template in the Synthesis of Cu-containing Nano/Submicro Particles
Author: ChenFangBo
Tutor: FangYun
School: Jiangnan University
Course: Applied Chemistry
Keywords: Sodium dodecyl sulfate Polyvinylpyrrolidone Bound micelle Cuprous oxide Hollow Submicrospheres Secondary self-assembly Copper nanoparticles Soft template
CLC: TB383.1
Type: Master's thesis
Year: 2007
Downloads: 62
Quote: 1
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Abstract
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In this paper , the anionic surfactant sodium dodecyl sulfate (SDS) , and water - soluble non-ionic macromolecular polyvinyl pyrrolidone (PVP) is formed soft cluster object of study, by the surface tension method and fluorescence quenching technique study with interaction , exploration of copper ions form a soft cluster structure of copper ions in the presence of SDS and PVP . Surface tension experiment showed that the addition of copper ions SDS is still bound to the micelle form with PVP clusters role of γ-lgc CuSO4 -SDS -PVP system curve remains double the critical concentration characteristics . Copper ion concentration increased beneficial SDS clusters PVP chain , so that the decrease of the surface tension γ strengthening , while C1 c2 increases decreases . The amount of saturated cluster Γ ∞ than the the the saturated cluster set amount of [Γ ∞] with the increase in the concentration of copper ions increases. The steady-state fluorescence quenching experiments results show that the the bound micelle aggregation number Nb with SDS concentration increases with the increase in the concentration of copper ions and reduce . N2H4 · H2O as reductant , SDS-PVP Soft Template restore the the CuSO4 preparation hollow Cu2O Submicrospheres . XRD patterns were determined by the average particle diameter of 11 ~ 22 nm of the original level Cu2O nanograins constitute mainly of (111) crystal face orientation . SEM and TEM experiments show that the resulting 420 ~ 550 nm structured hollow Cu2O Submicrospheres . SDS-PVP clusters like double soft template structure model successfully explained and a self-assembled the original level Cu2O nanocrystals synthesized in the the SDS bound micelles heavy template in the template in the second tier of the PVP stereo bridging secondary self-assembled secondary the hollow Cu2O Asia microspheres . Experimental facts indicate that SDS-PVP composite system , only the cluster -like structure is dominant only capable of inducing a synthetic the tacticity hollow Cu2O Submicrospheres ; adjustment cSDS can regulation within a certain range of the particle diameter of the hollow Cu2O Submicrospheres wall thickness and morphology . N2H4 · H2O restore the CuSO4 preparation of copper nanoparticles as a reducing agent in the SDS-PVP Soft Template . TEM and XRD experiments showed that the product of the average particle size of 20 ± 3 nm copper nanoparticles showed a face-centered cubic (fcc) structure . Combined with UV-Vis experiments shows that only when the SDS and PVP form a soft clusters exhibit particle morphology , size , superior regulation scale uniformity , dispersion and shape consistent nanoparticles .
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