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Preparation and Properties of Photoconductive Materials of Poly(2-(carbazol-9-yl) Ethyl Methacrylate)
Author: JiaLiXiang
Tutor: ZhangWenLong
School: Harbin University of Science and Technology
Course: Polymer Chemistry and Physics
Keywords: Poly ( methyl methacrylate ) N - vinyl carbazole Synthesis Characterization Photoconductive
CLC: O631.3
Type: Master's thesis
Year: 2011
Downloads: 17
Quote: 0
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Abstract
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The carbazoles polymer has excellent optical performance and hole conduction transmission performance , has broad application prospects in the energy , defense , information , health care , environmental protection, agriculture and other fields . Polyvinylcarbazole (PVK) because of their excellent photoconductive characteristics become best studied polymeric photoconductive material , but its presence high glass transition temperature , the film is poor , brittleness and other shortcomings , which greatly limits its research and application . This paper focuses on polymethacrylate ethylcarbazole acid ester (PCEM) , preparation methods , process conditions and photoconductive properties , lay the foundation for the research and application of new polymer photoconductive material . The transesterification method and nucleophilic substitution synthesis of methacrylic acid ethyl carbazole ester (CEM), the technological characteristics of the two kinds of preparation methods . The transesterification prepared CEM short time . The nucleophilic substitution prepared CEM post-processing is required chlorine ethylcarbazole readily available raw materials ( microwave synthesis ) . The microwave prepared chloroethyl carbazole process : stirring , the reaction temperature of 45 ° C , the reaction time was 40min , the microwave power is 600W . Microwave heating synthesis of chloro- ethyl carbazole than conventional heating short reaction time , low temperature , high yield . The conditions of preparation PCEM the system . Determine the preparation conditions : the CEM as raw materials , DMF as solvent , the reaction temperature was 85 ° C , reaction time 14h , initiator amount of the agent of AIBN 0.005g . By UV spectroscopy, infrared spectroscopy, NMR spectroscopy , gel permeation chromatography analysis method to characterize the synthesized product , and the PCEM studied by DSC and film . The results showed that : successfully synthesized a number average molecular weight of 2.9089 × 104g/mol PCEM , its glass transition temperature is 145.2 ° C , 40 ° C lower than PVK (185.4 ℃) has significantly improved deposition sexuality for PVK ; through the photoconductive test study PCEM photoelectric properties , compared with PVK . The analysis showed that: the PCEM the photoconductivity than PVK slightly higher under the same conditions , and the reaction temperature and reaction time to have a certain influence on the optical conductivity of the PCEM ; reaction time 14h , the reaction temperature was 85 ° C under PCEM photoconductivity a maximum of 5.469 × 10-18 S · cm -1 sup> .
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CLC: > Mathematical sciences and chemical > Chemistry > Polymer chemistry ( polymer ) > Polymer physics and physical chemistry of polymers > The chemical nature of polymers
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