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Synthesis and Research of LiFePO4/C as Cathode Material for Lithium Ion Battery
Author: ZhangGongZuo
Tutor: ChenGang
School: Harbin Institute of Technology
Course: Chemical Engineering and Technology
Keywords: Lithium ion battery Cathode material LiFePO4 / C Coated Doping
CLC: TM912.4
Type: Master's thesis
Year: 2007
Downloads: 246
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Abstract
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LiFePO 4 as a new lithium ion battery cathode materials with low prices, environmentally friendly, recycling and good performance. This article was prepared by carbothermal reduction LiFePO 4 / C, focuses on the different amount of sugar added and doping Mg 2 sup> on the prepared LiFePO 4 sub > crystal structure and properties. By powder X-ray diffraction method (X-ray Diffraction, XRD), Fourier transform - infrared spectroscopy (Fourier Transform Infrared, FT-IR), scanning electron microscope (Scanning Electron Microscope, SEM), constant current charge and discharge, cyclic voltammetry security and other means of LiPePO 4 phase structure, morphology and electrochemical properties were analyzed. In LiNO 3 , Fe (NO 3 ) 3 · 9H 2 O, NH 4 H 2 PO 4 and C 12 H 22 O 11 for raw materials by carbothermal reduction method synthetic samples, XRD analysis showed that the synthesized samples olivine LiFePO 4 . By FT-IR and SEM analysis showed that the carbon-coated LiFePO 4 around and found that the amount of sugar added to increase the carbon-coated LiFePO 4 of volume increase, carbon-coated layer has a thickness of about 20nm. Cycle performance tests show that the amount of sugar added 63mass%, the best performance of the sample loop, 0.1C current maximum discharge capacity of 143.2mAh / g, 2C current discharge capacity of 99.8mAh / g. After doing 2C current cycle 40 times, do 0.1C current cycle performance test and found that the first discharge capacity of 137.5mAh / g, the specific capacitance of the sample has a good recovery. Sucrose addition is 63mass% of the samples were doped with Mg 2 sup> modified, XRD analysis showed that the synthesized samples olivine-type LiFePO 4 . As doping increases, the diffraction peaks shifted to higher angles, indicating Mg 2 sup> substituted LiFePO 4 in the part of Fe 2 sup>. SEM detected, doping did not have an impact on the carbon coating layer. Mg doping of 0.05, that LiMg 0.05 Fe 0.95 PO 4 / C cycle performance is better. 0.1C current initial discharge capacity of 122.1mAh / g, 2C current initial discharge capacity of 88.7mAh / g. Carbothermal reduction method using synthetic samples with a simple process, low price of LiFePO 4 electrochemical performance improvement effect is obvious in the commercialization of LiFePO 4 has a good potential applications.
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CLC: > Industrial Technology > Electrotechnical > Independent power supply technology (direct power) > Battery > Sealed battery
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