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Studies on Syntheses of Precious Metal Nanoclusters and Their Catalytic and Magnetic Properties
Author: YangLiPing
Tutor: WangWenChuanï¼›TuWeiXia
School: Beijing University of Chemical Technology
Course: Chemical Engineering
Keywords: Nano - metal clusters Microwave radiation Preparation Catalytic properties Magnetic properties
CLC: O643.32
Type: Master's thesis
Year: 2006
Downloads: 194
Quote: 1
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Abstract
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This paper studies the synthesis and catalytic metal clusters of nanometer consistent , magnetic properties , including the following : 1) the use of chemical reduction synthesis of polyvinylpyrrolidone (PVP) stable , non - supported palladium / iron oxide nano metal colloidal clusters and load type Pd / Fe 2 O 3 , Pd / Fe 3 O 4 and Pd-Pt/Fe 3 O 4 nano - metal clusters , and transmission electron microscopy ( TEM ) , vibrating sample magnetometer (VSM) with its characterization . Resulting Pd / Fe 3 O 4 and Pd-Pt/Fe 3 O 4 sample with magnetic With easy recovery of advantages to the magnetic field in the selective hydrogenation of o-chloronitrobenzene reaction showed better catalytic performance than Pd and Pd-Pt nano - metal clusters and reusability . 2 ) Prepared by Microwave the PVP stability of gold colloid particles , effects of alcohol reducing agent as well as alkali gold particles formed were characterized using a transmission electron microscope , UV - visible spectrophotometer . The results showed that the microwave prepared gold colloidal particles with a small particle size , good dispersion . The size and shape of the gold particles with different alcohol the kind of the reducing agent and an alkali NaOH dosage , there are significant changes . UV - visible absorption spectra showed that the faster the system of adding an alkali in the reaction mixture , the rate of formation of the gold particles were significantly higher than not adding an alkali , and is conducive to the formation of spherical gold particles . 3) synthesized by chemical reduction method organic molecular layer ( Octadecanethiol ) is protected palladium and palladium / iron oxide , metal clusters , the obtained nano - particles have an average particle size of about 1.5nm . Research
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CLC: > Mathematical sciences and chemical > Chemistry > Physical Chemistry ( theoretical chemistry ),chemical physics > Chemical kinetics,catalysis > Catalytic > Catalytic reaction
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